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CHEM 5623: Physical Chemistry III: Quantum Chemistry

Syllabus
Location and time: Bizzell library, room 418 (Tue and Thur 1:30-2:45 pm)
Office hour: Thur 3:00-5:30 pm or by appointment (CHB 309)

Schedule (subject to change)

Dates Topics Reading Lecture notes

Week 1
8/26, 8/28 

Particle-wave duality, origin of Schrodinger equation, particle in a one-dimensional box, uncertainty principle

Levine, Chap. 1, 2

Notes 1, Notes 2,
Problem set 1

Week 2
 9/2, 9/4

Operators, Hamilton mechanics, harmonic oscillator, commutators, simultaneous determination of two properties

Levine, Chap. 3, 4

Notes 3, Notes 4,
Problem set 2

Week 3
9/9, 9/11

Angular momentum, ladder operator method

Levine, Chap. 5

Notes 5, Notes 6,
Problem set 3

Week 4
9/16, 9/18

Rigid rotor, hydrogen atom

Levine, Chap. 6

Notes 7, Notes 8, Problem set 4

Week 5
9/23, 9/25

Eigenfunctions, operators, measurement outcomes, postulates

Levine, Chap. 7

Notes 9, Notes 10, Problem set 5

Week 6
9/30, 10/2

Matrices, determinants, complex vector space,
change of basis, eigenvalue problem

Szabo, Chap. 1

Notes 11, Notes 12,
Problem set 6

Week 7
10/7, 10/9

Function of matrices, function space and vector space, mid-term exam

 Szabo, Chap. 1

Notes 13

Week 8
10/14, 10/16

Variation theorem, linear variation method, perturbation theory

Levine, Chap. 8, 9

Notes 14, Notes 15,
Problem set 7

Week 9
10/21, 10/23

Spin angular momentum, Fermions and Bosons, spin orbitals, Slater determinant wave function

Levine, Chap. 10; Szabo Chap. 2.2

Notes 16, Notes 17
Problem set 8

Week 10
10/28, 10/30

Born-Oppenheimer approximation, Intro to Hartree-Fock and CI theory, angular momentum for many-electron atoms

Szabo Chap. 2.1, 2.2; Levine, Chap. 11

Notes 18, Notes 19
Problem set 9

Week 11
11/4, 11/6

One- and two-electron integrals, CI matrix elements

Szabo Chap. 2.3

Notes 20, Notes 21
Problem set 10

Week 12
11/11, 11/13

Spin-adapted configurations, derivation of HF equation

Szabo, Chap. 2.5, 3.1, 3.2

Notes 22, Notes 23
Problem set 11

Week 13
11/18, 11/20

Koopman theorem, restricted and unrestricted HF, restricted closed-shell HF: Roothaan equations

Szabo, Chap. 3.3, 3.4

Notes 24, Notes 25

Week 14
11/25

SCF, dipole moment, population analysis, basis functions

Szabo, Chap. 3.4

Notes 26
Problem set 12

Week 15
12/2, 12/4

Bond order, localized MO, Pople-Nesbet equations, Density functional theory

Szabo 3.8

Notes 27, Notes 28
Problem set 13

Week 16
12/9, 12/11

Empirical DFT theory, virial theorem, review

Levine, Chap. 14

Notes 29
Week 17
12/17
final exam